A 2010 Draft Pick, Kole Calhoun first made the majors with the Los Angeles Angels in 2012, becoming a starter at baseball’s highest level in 2014 at Rightfield.  

In his first full season, Calhoun batted .272 with 17 Home Runs, and he followed that with back-to-back 161 Hit Years, which again had at least double-digit power numbers.  Winning a Gold Glove in 2015, Calhoun kept his power numbers respectable, though he never matched his .272 Batting Average in 2014.  In 2019, which would be his last year as an Angel (he signed with Arizona after), he smashed 33 Home Runs.

With the Angels, Calhoun had 884 Hits with 140 Home Runs. 

Don Baylor joined Anaheim in 1977 as a key signing during the early free-agency period. He was a muscular slugger whose presence marked a bold new era for the team. Although he is now well-known for his later roles as a manager and hitting coach, his playing days in California were characterized by a particular kind of power-driven middle-of-the-order intimidation.

Baylor’s 1979 season is among the most successful in the team's history. That summer, he proved his skill in driving in runs at an exceptional pace, leading the American League with 139 RBIs and scoring 120 runs. He demonstrated his elite status by hitting 36 home runs and earning the 1979 American League MVP, becoming the first in franchise history to receive the award. This consistent production was the key factor that helped the Angels reach their first postseason. Interestingly, it also marked his only All-Star appearance in a Halos uniform.

Known for "crowding the plate" and standing firm, he led the league twice in hit-by-pitches. From 1977 to 1982, he demonstrated consistent power, averaging nearly 24 home runs annually despite missing much of 1980 due to a major injury. Although he was a key run-producer, his overall value was limited by particular difficulties in the field.  Bluntly, he was a defensive liability throughout his stay with the Angels.

After 141 home runs and over 500 RBIs, Baylor departed for the New York Yankees as a free agent. In 1990, he was inducted into the Angels Hall of Fame, becoming just the third man to receive the honor.

Ervin Santana joined the California organization as an amateur free agent in 2000. This Dominican right-hander was known for his powerful fastball and slider, which were expected to be the backbone of the rotation for years. He made his debut in 2005, quickly fitting into a clubhouse fresh off a world title and showing signs of a top-tier starter. Over eight seasons with the Angels, he displayed a unique lot of "feast or famine" dominance, indicating that although he lacked consistent performance, his raw talent could overpower any lineup.

In his first two summers in the rotation, he established himself as a dependable key player, posting a 12-8 rookie record, which he improved to 16 wins in 2006. His career hit a setback in 2007 due to technical problems and a demotion to the minors. Showing resilience, he made a remarkable comeback in 2008, his best season with Anaheim. That year, he had 16 wins, achieved a career-high 214 strikeouts, and earned his first All-Star selection, finishing sixth in Cy Young Award voting.

His time in Orange County was marked by fluctuations over the next four years. He frequently pitched deep into games, highlighted by a career-high 17 wins in 2010, but he also faced seasons where his ERA rose above 5. Despite these ups and downs, he achieved a historic individual moment on July 27, 2011, when he threw a no-hitter against the Cleveland Indians.

In October 2012, he was traded to the Kansas City Royals as the team looked to reshuffle its pitching staff. With the Angels, Santana had a 96-80 record with a 4.33 ERA and 1,167 strikeouts.

In December 2011, Albert Pujols arrived in Anaheim with a ten-year, $240 million contract, aiming to reshape the American League's power dynamics. Already a first-ballot Hall of Famer after a decade of record-breaking performance in St. Louis, he brought high expectations to the Angels' roster. Over nearly ten seasons in Southern California, he offered a unique veteran power, chasing historic baseball milestones. However, his time there ultimately became a stark reminder of athletic decline.

In 2012, he showcased his ability to succeed on the Junior Circuit, hitting 30 home runs and collecting 105 RBIs while maintaining a .285 batting average. He demonstrated his professionalism as a run-producer with a strong 2015 season, hitting 40 home runs and earning his only All-Star selection as a Halo. This consistent power threat served as a key element in the lineup during the club’s 98-win season in 2014, offering a veteran presence alongside a young Mike Trout.

Over time, his stint in Orange County was increasingly marked by a decline in his secondary skills. As years passed, his technical hitting ability was gradually diminished by reduced mobility and a declining on-base percentage. While he demonstrated his value to the organization by recording over 100 RBIs in four seasons, these strong stats often concealed a decline in overall effectiveness; as his fielding range diminished and his speed waned, his advanced metrics also dropped sharply. By the late 2010s, he found it difficult to reach a .300 on-base percentage, and his bWAR frequently turned negative, indicating a decline from his former status as one of the most complete hitters in the game.

In May 2021, when the franchise aimed to cut his playing time to give more opportunities to younger players, a specific disagreement resulted in his release. This marked the end of a tenure that was as much defined by a burdensome contract as by his legendary home runs.

While his contract might have been cumbersome to the Angels, Pujols still compiled 1,180 hits and 222 home runs.